{"id":461,"date":"2025-03-13T16:57:33","date_gmt":"2025-03-13T15:57:33","guid":{"rendered":"https:\/\/staging-scf.agence-nsw.xyz\/chimie-de-coordination\/actualites\/prix-de-these-2024\/"},"modified":"2025-03-13T16:57:33","modified_gmt":"2025-03-13T15:57:33","slug":"prix-de-these-2024","status":"publish","type":"post","link":"https:\/\/staging-scf.agence-nsw.xyz\/chimie-de-coordination\/fr\/actualites\/prix-de-these-2024\/","title":{"rendered":"Prix de th\u00e8se 2024"},"content":{"rendered":"\n<p class=\"wp-block-paragraph\">Le bureau de la DCC s\u2019est r\u00e9uni pour l\u2019attribution du <strong>prix de th\u00e8se 2024<\/strong>. Nous avons re\u00e7u des candidatures de tr\u00e8s grande qualit\u00e9, illustrant la chimie de coordination dans toute sa diversit\u00e9. Nous tenons \u00e0 f\u00e9liciter toutes les candidates pour leur fort engagement dans leur projet de doctorat.<\/p>\n\n\n\n<p class=\"wp-block-paragraph\"><img decoding=\"async\" class=\"wp-image-214963\" style=\"width: 150px\" src=\"https:\/\/new.societechimiquedefrance.fr\/wp-content\/uploads\/2025\/03\/Sara-Bonfante-1.jpg\" alt=\"\"><\/p>\n\n\n\n<p class=\"wp-block-paragraph\">Le prix de th\u00e8se DCC 2024 a \u00e9t\u00e9 attribu\u00e9 \u00e0\u00a0<strong>Sara Bonfante <\/strong>pour ses travaux intitul\u00e9s\u00a0<strong><em>Zirconium- and Phosphine-Assisted C\u2013F Bond Activation and Functionalisation<\/em><\/strong>, men\u00e9s au Laboratoire de chimie de coordination (LCC) de l&rsquo;Universit\u00e9 de Toulouse III, Paul Sabatier, et \u00e0 l&rsquo;Universit\u00e9 de York au Royaume-Uni, sous la supervision des Dr Antoine Simonneau, Dr John Slattery, Prof Jason Lynam et Dr Christian Lorber.<\/p>\n\n\n\n<p class=\"wp-block-paragraph\">L&rsquo;objectif de cette recherche de doctorat \u00e9tait de d\u00e9velopper de nouveaux protocoles st\u0153chiom\u00e9triques et catalytiques pour la <strong>fonctionnalisation r\u00e9gios\u00e9lective de la liaison C-F d&rsquo;aromatiques polyfluor\u00e9s<\/strong>.<\/p>\n\n\n\n<p class=\"wp-block-paragraph\">Le projet a d&rsquo;abord d\u00e9montr\u00e9 que l&rsquo;inversion de polarit\u00e9, ou \u00ab umpolung \u00bb, du cyclohexyne, obtenue par complexation avec le zirconoc\u00e8ne, rendait le petit cycloalkyne d\u00e9form\u00e9 apte \u00e0 la fonctionnalisation de la liaison C-F des fluoropyridines [1]. Cette forte activation de la liaison chimique est sans pr\u00e9c\u00e9dent dans la chimie des arynes \u00ab libres \u00bb et des alcynes d\u00e9form\u00e9s. L&rsquo;\u00e9tude a \u00e9galement montr\u00e9 que la r\u00e9activit\u00e9 du complexe Zr-cyclohexyne d\u00e9pendait fortement du degr\u00e9 de fluoration de l&rsquo;h\u00e9t\u00e9roar\u00e8ne. La r\u00e9activit\u00e9 inattendue impliquant le ligand phosphine a conduit au d\u00e9veloppement d&rsquo;une nouvelle direction de recherche, explorant la r\u00e9activit\u00e9 de la phosphine avec les aromatiques fluor\u00e9s.<\/p>\n\n\n\n<p class=\"wp-block-paragraph\">Cette recherche a d\u00e9montr\u00e9 que la catalyse m\u00e9tallomim\u00e9tique, impliquant un cycle redox entre les \u00e9tats d&rsquo;oxydation P(III) et P(V), est r\u00e9alisable en utilisant uniquement des trialkylphosphines simples et peu co\u00fbteuses telles que PnBu3, sans n\u00e9cessiter de g\u00e9om\u00e9tries complexes ou d&rsquo;agents oxydants\/r\u00e9ducteurs externes [2]. Les r\u00e9actions d&rsquo;hydrod\u00e9fluoration et d&rsquo;aminod\u00e9fluoration d&rsquo;une vari\u00e9t\u00e9 de fluoroar\u00e8nes ont \u00e9t\u00e9 r\u00e9alis\u00e9es avec succ\u00e8s dans des conditions douces, avec des rendements bons \u00e0 excellents. <strong>Ces r\u00e9sultats ouvrent un nouveau champ de recherche sur les fonctionnalisations catalys\u00e9es par les phosphines, avec une large applicabilit\u00e9 dans les milieux acad\u00e9miques et industriels.<\/strong><\/p>\n\n\n\n<p class=\"wp-block-paragraph\">[1] <a href=\"https:\/\/pubs.rsc.org\/en\/content\/articlelanding\/2025\/sc\/d4sc08522a\">S. Bonfante, C. Lorber, J. M. Lynam, A. Simonneau, J. M. Slattery, <em>Chem. Sci.<\/em> <strong>2025<\/strong>, <em>16<\/em>, 3552\u20133559.<\/a><\/p>\n\n\n\n<p class=\"wp-block-paragraph\">[2] <a href=\"https:\/\/pubs.acs.org\/doi\/10.1021\/jacs.3c10614\">S. Bonfante, C. Lorber, J. M. Lynam, A. Simonneau, J. M. Slattery, <em>J. Am. Chem. Soc<\/em>. <strong>2024<\/strong>, <em>146<\/em>, 3, 2005\u20132014.<\/a><\/p>\n\n\n\n<p class=\"wp-block-paragraph\"><\/p>\n","protected":false},"excerpt":{"rendered":"<p>Le bureau de la DCC s\u2019est r\u00e9uni pour l\u2019attribution du prix de th\u00e8se 2024. Nous avons re\u00e7u des candidatures de tr\u00e8s grande qualit\u00e9, illustrant la chimie de coordination dans toute sa diversit\u00e9. Nous tenons \u00e0 f\u00e9liciter toutes les candidates pour leur fort engagement dans leur projet de doctorat. Le prix de th\u00e8se DCC 2024 a [&hellip;]<\/p>\n","protected":false},"author":3,"featured_media":0,"comment_status":"open","ping_status":"open","sticky":false,"template":"","format":"standard","meta":{"_acf_changed":false,"footnotes":""},"categories":[1],"tags":[],"class_list":["post-461","post","type-post","status-publish","format-standard","hentry","category-actualites"],"acf":[],"yoast_head":"<!-- This site is optimized with the Yoast SEO plugin v28.7 - https:\/\/yoast.com\/product\/yoast-seo-wordpress\/ -->\n<title>Prix de th\u00e8se 2024 - SCF Division Chimie de coordination<\/title>\n<meta name=\"robots\" content=\"noindex, follow, max-snippet:-1, max-image-preview:large, max-video-preview:-1\" \/>\n<meta property=\"og:locale\" content=\"fr_FR\" \/>\n<meta property=\"og:type\" content=\"article\" \/>\n<meta property=\"og:title\" content=\"Prix de th\u00e8se 2024 - SCF Division Chimie de coordination\" \/>\n<meta property=\"og:description\" content=\"Le bureau de la DCC s\u2019est r\u00e9uni pour l\u2019attribution du prix de th\u00e8se 2024. Nous avons re\u00e7u des candidatures de tr\u00e8s grande qualit\u00e9, illustrant la chimie de coordination dans toute sa diversit\u00e9. Nous tenons \u00e0 f\u00e9liciter toutes les candidates pour leur fort engagement dans leur projet de doctorat. 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