{"id":454,"date":"2024-03-06T20:30:54","date_gmt":"2024-03-06T19:30:54","guid":{"rendered":"https:\/\/staging-scf.agence-nsw.xyz\/chimie-de-coordination\/actualites\/prix-de-these-2023\/"},"modified":"2024-03-06T20:30:54","modified_gmt":"2024-03-06T19:30:54","slug":"prix-de-these-2023","status":"publish","type":"post","link":"https:\/\/staging-scf.agence-nsw.xyz\/chimie-de-coordination\/fr\/actualites\/prix-de-these-2023\/","title":{"rendered":"Prix de th\u00e8se 2023"},"content":{"rendered":"\n<p class=\"wp-block-paragraph\">Le bureau de la DCC s\u2019est r\u00e9uni pour l\u2019attribution du <strong>prix de th\u00e8se 2023<\/strong>. Nous avons re\u00e7u des candidatures de tr\u00e8s grande qualit\u00e9, illustrant la chimie de coordination dans toute sa diversit\u00e9. Nous tenons \u00e0 f\u00e9liciter tous les candidats pour leur fort engagement dans leur projet de doctorat.<\/p>\n\n\n\n<div class=\"wp-block-columns is-layout-flex wp-container-core-columns-is-layout-7387b849 wp-block-columns-is-layout-flex\">\n<div class=\"wp-block-column is-layout-flow wp-block-column-is-layout-flow\">\n<figure class=\"wp-block-image size-large is-resized\"><img loading=\"lazy\" decoding=\"async\" src=\"https:\/\/new.societechimiquedefrance.fr\/wp-content\/uploads\/2024\/03\/IMG-20240229-WA00002-819x1024.jpg\" alt=\"\" class=\"wp-image-202610\" width=\"322\" height=\"401\" \/><\/figure>\n<\/div>\n\n\n\n<div class=\"wp-block-column is-layout-flow wp-block-column-is-layout-flow\">\n<p class=\"wp-block-paragraph\"> <\/p>\n\n\n\n<p class=\"wp-block-paragraph\">                                                              Le prix de th\u00e8se DCC 2023 a \u00e9t\u00e9 attribu\u00e9 \u00e0 <strong><span class=\"has-inline-color has-vivid-red-color\">Eva Pugliese<\/span><\/strong> pour ses travaux intitul\u00e9s <strong><em><span class=\"has-inline-color has-vivid-cyan-blue-color\">Photocatalyse mol\u00e9culaire pour l&rsquo;activation de petites mol\u00e9cules<\/span><\/em><\/strong>, sous la direction du Prof. Ally Aukauloo et la codirection du Dr. Zakaria Halime, travaux de recherche men\u00e9s \u00e0 l&rsquo;Institut d&rsquo;Orsay de Chimie Mol\u00e9culaire et des Mat\u00e9riaux de l&rsquo;Universit\u00e9 Paris-Saclay.<\/p>\n\n\n\n<p class=\"wp-block-paragraph\">Le prix (accompagn\u00e9 de la somme de 300 \u20ac) sera remis \u00e0 Eva lors des prochaines <strong><span class=\"has-inline-color has-vivid-cyan-blue-color\">Journ\u00e9es de Chimie de Coordination 2025<\/span><\/strong> \u00e0 Orsay, o\u00f9 nous aurons le plaisir de l\u2019\u00e9couter lors d\u2019une communication orale sur son travail de th\u00e8se.<\/p>\n<\/div>\n<\/div>\n\n\n\n<p class=\"wp-block-paragraph\"><strong>Toutes nos f\u00e9licitations !<\/strong><\/p>\n\n\n\n<p class=\"wp-block-paragraph\">Le grand d\u00e9fi de son travail de doctorat \u00e9tait d&rsquo;apporter une compr\u00e9hension approfondie du <strong><span class=\"has-inline-color has-vivid-red-color\">cycle photocatalytique de r\u00e9duction du CO<sub>2<\/sub> en CO <\/span><\/strong>induit par la lumi\u00e8re en utilisant le m\u00e9lange d&rsquo;une porphyrine de fer con\u00e7ue comme catalyseur, d&rsquo;un photosensibilisateur et d&rsquo;un donneur d&rsquo;\u00e9lectrons sacrificiel. Il est important de mentionner que diff\u00e9rentes propositions figuraient d\u00e9j\u00e0 dans la litt\u00e9rature, mais sans aucune preuve spectroscopique de la pr\u00e9sence d&rsquo;interm\u00e9diaires. Mme Pugliese a synth\u00e9tis\u00e9 et \u00e9tudi\u00e9 l&rsquo;activit\u00e9 photocatalytique d&rsquo;une porphyrine de fer flanqu\u00e9e de groupes ur\u00e9e pour servir d&rsquo;\u00e9chafaudage \u00e0 des liaisons hydrog\u00e8ne en deuxi\u00e8me sph\u00e8re de coordination. Elle a r\u00e9alis\u00e9 en parall\u00e8le des \u00e9tudes spectro\u00e9lectrochimiques et photophysiques pour prouver que c&rsquo;est l&rsquo;esp\u00e8ce Fe(I) qui est l&rsquo;\u00e9tat stable et que l&rsquo;\u00e9tape limitante est la coordination du CO<sub>2<\/sub> sur l\u2019esp\u00e8ce de Fe(I), r\u00e9sultats qui marquent un changement de paradigme dans l\u2019activation du CO<sub>2<\/sub> [1]. Capitalisant sur les propri\u00e9t\u00e9s extraordinaires de la porphyrine de fer pr\u00e9c\u00e9demment \u00e9tudi\u00e9e, elle s\u2019est attel\u00e9e ensuite \u00e0 la conception d\u2019une photocathode pour r\u00e9duire le CO<sub>2<\/sub> en solution aqueuse.<\/p>\n\n\n\n<p class=\"wp-block-paragraph\">En parall\u00e8le, elle a abord\u00e9 l\u2019<strong><span class=\"has-inline-color has-vivid-red-color\">oxydation d\u2019alc\u00e8nes par le dioxyg\u00e8ne<\/span><\/strong> gr\u00e2ce \u00e0 un catalyseur \u00e0 base de fer qui est activ\u00e9 par absorption de la lumi\u00e8re via un photosensibilisateur. Elle a \u00e9tudi\u00e9 les m\u00e9canismes complexes de la photocatalyse mol\u00e9culaire et a identifi\u00e9 les esp\u00e8ces photog\u00e9n\u00e9r\u00e9es fer-hydroperoxo et fer-peroxo caract\u00e9ris\u00e9es par spectroscopie UV-vis et RPE, \u00e9cartant tout doute sur un m\u00e9canisme radicalaire cach\u00e9 [2].<\/p>\n\n\n\n<p class=\"wp-block-paragraph\">[1] <a href=\"https:\/\/onlinelibrary.wiley.com\/doi\/10.1002\/anie.202117530\" target=\"_blank\" rel=\"noreferrer noopener\">E. Pugliese, P. Gotico, I. Wehrung, B. Boitrel, A. Quaranta, M.-H. Ha-Thi, T. Pino, M. Sircoglou, W. Leibl, Z. Halime, A. Aukauloo, Dissection of Light-Induced Charge Accumulation at a Highly Active Iron Porphyrin: Insights in the Photocatalytic CO<sub>2<\/sub> Reduction, <em>Angew. Chem. Int. Ed.<\/em> <strong>2022<\/strong>, 61, e202117530.<\/a><br>[2] <a href=\"https:\/\/pubs.rsc.org\/en\/content\/articlelanding\/2022\/sc\/d2sc03129a\" target=\"_blank\" rel=\"noreferrer noopener\">E. Pugliese, N. T. Vo, A. Boussac, F. Banse, Y. Mekmouche, J. Simaan, T. Tron, P. Gotico, M. Sircoglou, Z. Halime, W. Leibl, A. Aukauloo, Photocatalytic generation of a non-heme Fe(iii)-hydroperoxo species with O<sub>2<\/sub> in water for the oxygen atom transfer reaction, <em>Chem. Sci. <\/em><strong>2022<\/strong>, 13, 12332-12339.<\/a><\/p>\n","protected":false},"excerpt":{"rendered":"<p>Le bureau de la DCC s\u2019est r\u00e9uni pour l\u2019attribution du prix de th\u00e8se 2023. Nous avons re\u00e7u des candidatures de tr\u00e8s grande qualit\u00e9, illustrant la chimie de coordination dans toute sa diversit\u00e9. Nous tenons \u00e0 f\u00e9liciter tous les candidats pour leur fort engagement dans leur projet de doctorat. Le prix de th\u00e8se DCC 2023 a [&hellip;]<\/p>\n","protected":false},"author":3,"featured_media":0,"comment_status":"open","ping_status":"open","sticky":false,"template":"","format":"standard","meta":{"_acf_changed":false,"footnotes":""},"categories":[1],"tags":[],"class_list":["post-454","post","type-post","status-publish","format-standard","hentry","category-actualites"],"acf":[],"yoast_head":"<!-- This site is optimized with the Yoast SEO plugin v28.7 - https:\/\/yoast.com\/product\/yoast-seo-wordpress\/ -->\n<title>Prix de th\u00e8se 2023 - SCF Division Chimie de coordination<\/title>\n<meta name=\"robots\" content=\"noindex, follow, max-snippet:-1, max-image-preview:large, max-video-preview:-1\" \/>\n<meta property=\"og:locale\" content=\"fr_FR\" \/>\n<meta property=\"og:type\" content=\"article\" \/>\n<meta property=\"og:title\" content=\"Prix de th\u00e8se 2023 - SCF Division Chimie de coordination\" \/>\n<meta property=\"og:description\" content=\"Le bureau de la DCC s\u2019est r\u00e9uni pour l\u2019attribution du prix de th\u00e8se 2023. Nous avons re\u00e7u des candidatures de tr\u00e8s grande qualit\u00e9, illustrant la chimie de coordination dans toute sa diversit\u00e9. Nous tenons \u00e0 f\u00e9liciter tous les candidats pour leur fort engagement dans leur projet de doctorat. 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